Quantum geometry of materials mapped with light, researchers say

Image: Universität Jena · uni-jena.de

Researchers at Friedrich Schiller University Jena and the University of Regensburg have demonstrated a new optical technique for quantifying Berry curvature, a quantum property influencing electron behavior, within a single atomic layer of tungsten diselenide. The team used ultrashort laser pulses to measure the curvature, a feat previously accomplished only through complex experimental methods.

“We wanted to make a quantum property accessible that has so far been difficult to determine experimentally,” says lead author Nele Tornow of the University of Jena’s Institute of Solid State Physics. Published in the latest issue of Nature Photonics, the method combines optical measurements with an analytical model to reveal these subtle quantum geometric properties.

Nonlinear Circular Dichroism Reveals Quantum Geometric Properties

Researchers directed ultrashort laser pulses at this material, demonstrating the technique’s capability at an extremely small scale and opening a new avenue for investigating quantum geometry. The measurement relies on a two-pulse sequence; the first alters the material’s electronic states for a minuscule fraction of a second, while the second detects this change optically. This interaction generates light at twice the frequency of the initial laser, and the polarisation of this emitted light reveals information about the Berry curvature.

The entire process occurs within a few hundred femtoseconds, a unit of time representing one millionth of a billionth of a second, highlighting the speed at which these quantum properties can be probed. Changing the rotation direction of the initial laser pulse reverses the sign of the measured signal, providing a clear indicator of the curvature.

The team’s approach provides a specific value for the Berry curvature, a significant improvement over previous methods that primarily relied on theoretical calculations or complex experimental setups. The measured Berry curvature aligned with theoretical calculations, validating the accuracy of the new optical technique and its analytical model.

Giancarlo Soavi from the Institute of Solid State Physics and the Abbe Centre of Photonics at the University of Jena explains that this optical method allows investigation of these properties on extremely short timescales. The team states that the fundamental principles of their method are applicable to other materials, suggesting a broader potential for mapping quantum geometric properties, and the analytical model, developed in collaboration with researchers from the University of Regensburg, is designed to be adaptable, further expanding the technique’s reach.

The first pulse alters the electronic states of the material for a tiny fraction of a second.

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Ivy Delaney

Ivy Delaney has been working with neural networks and machine learning since the mid-nineties, back when a couple of hidden layers and a long afternoon of training counted as ambitious. She has watched the field go from academic curiosity to the thing quietly running underneath everything, and she brings that long view to quantum computing. For Quantum Zeitgeist she covers the ground where the two fields meet. That means quantum machine learning and the variational algorithms it leans on, and it also means the less glamorous but more interesting story of classical machine learning already doing real work inside quantum machines, decoding error-correcting codes, calibrating noisy hardware and learning the error models that simulators depend on. She writes about the hardware those algorithms have to run on too, and about the post-quantum cryptography scramble that the same hardware has set off. Her stories typically start with the paper, whether that is peer-reviewed work, conference proceedings or an arXiv preprint, with the source linked so you can hold a claim up against the research it came from. She is unimpressed by benchmarks that will not say what they beat, and by demonstrations that only work in the press release.

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